Date: Dec. 8^th to Dec. 12^th 2014 (more)

Phys. Rev. X 4, 041019 (2014)
We perform systematic investigations of transport through graphene on hexagonal boron nitride (hBN) substrates, together with confocal Raman measurements and a targeted theoretical analysis, to identify the dominant source of disorder in this system. (more)

Physica Status Solidi B (online)
We present Raman spectroscopy measurements of non-etched graphene nanoribbons, with widths ranging from 15 to 160 nm, where the D-line intensity is strongly dependent on the polarization direction of the incident light. The extracted edge disorder correlation length is approximately one order of magnitude larger than on previously reported graphene ribbons fabricated by reactive ion etching techniques. This suggests a more regular crystallographic orientation of the non-etched graphene ribbons here presented. We further report on the ribbons width dependence of the line-width and frequency of the long-wavelength optical phonon mode (G-line) and the 2D-line in the studied graphene ribbons.

Nano Lett. 14, 6050 (2014)
We present a new fabrication method of graphene spin-valve devices that yields enhanced spin and charge transport properties by improving both the electrode-to-graphene and graphene-to-substrate interface. First, we prepare Co/MgO spin injection electrodes onto Si⁺⁺/SiO₂. Thereafter, we mechanically transfer a graphene–hBN heterostructure onto the prepatterned electrodes. We show that room temperature spin transport in single-, bi-, and trilayer graphene devices exhibit nanosecond spin lifetimes with spin diffusion lengths reaching 10 μm combined with carrier mobilities exceeding 20,000 cm²/(Vs).

Phys. Rev. B 90, 165403 (2014)
By successive oxygen treatments of graphene nonlocal spin-valve devices we achieve a gradual increase of the contact-resistance–area products (R_cA) of Co/MgO spin injection and detection electrodes and a transition from linear to nonlinear characteristics in the respective differential dV−dI curves. With this manipulation of the contacts, both spin lifetime and the amplitude of the spin signal can significantly be increased by a factor of seven in the same device. This demonstrates that contact-induced spin dephasing is the bottleneck for spin transport in graphene devices with small R_cA values. With increasing R_cA values, we furthermore observe the appearance of a second charge neutrality point (CNP) in gate-dependent resistance measurements. Simultaneously, we observe a decrease of the gate voltage separation between the two CNPs. The strong enhancement of the spin-transport properties as well as the changes in charge transport are explained by a gradual suppression of a Co-graphene interaction by improving the oxide barrier during oxygen treatment.